Sources and Flux of Dissolved Inorganic Carbon in the Hydrothermally Active Corner of a Backarc Basin (Southwestern Okinawa Trough)
Journal
Journal of Geophysical Research: Oceans
Journal Volume
129
Journal Issue
6
ISSN
2169-9275
2169-9291
Date Issued
2024-06
Author(s)
Lin, Yu‐Shih
Huang, Wei‐Jen
Lan, Tefang
Shao, Huan‐Jie
Fu, Ke‐Hsien
Lee, Hsiao‐Fen
Wang, Bo‐Shian
Takahata, Naoto
Sano, Yuji
Chen, Song‐Chuen
Wang, Yunshuen
Lee, I‐Huan
Abstract
CO2 released from subduction zones plays a vital role in the tectonic carbon cycle. However, the contribution of submarine backarc components to carbon emissions remains poorly understood compared to subaerial arc volcanos. This study utilized a combination of geochemical and hydrodynamic approaches to investigate the sources and flux of dissolved inorganic carbon (DIC) in the deep basin of the southwestern Okinawa Trough. Most deep-water (depth ≥1,000 m) samples, even those retrieved from sites distant from active venting, exhibited mild geochemical anomalies of elevated 3He/4He ratios and higher DIC content than reference sites. Hydrodynamic observations using bottom-mounted acoustic instruments in the deep basin revealed strong tidal currents and enhanced turbulent mixing. These findings suggest that active solute dispersal and mixing are responsible for the prevalence of mild geochemical anomalies in the basin. Mixing models indicated that hydrothermal vent fluids are the primary source of excess 3He and DIC above background levels in the deep basin, whereas both CO2 and mineral acid in hydrothermal fluids cause excess acidity. Based on hydrodynamic and geochemical data, a box model estimated a hydrothermal DIC flux of 0.62 ± 1.40 × 1010 mol y−1, equivalent to 40% of CO2 emissions from persistently degassing volcanos in the Ryukyu Arc. Our results suggest that submarine carbon emissions are quantitatively important in subduction systems with subaqueous backarc components.
Subjects
backarc basin
carbon flux
hydrothermalism
Okinawa Trough
Publisher
American Geophysical Union (AGU)
Type
journal article