Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases
Journal
Chemical Physics Letters
Journal Volume
189
Journal Issue
4-5
Pages
346-352
Date Issued
1992
Author(s)
Abstract
Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation. © 1992.
Type
journal article