https://scholars.lib.ntu.edu.tw/handle/123456789/598219
標題: | Machine Learning with Explainable Artificial Intelligence Vision for Characterization of Solution Conductivity Using Optical Emission Spectroscopy of Plasma in Aqueous Solution | 作者: | Wang C.-Y Ko T.-S Hsu C.-C. JERRY CHENG-CHE HSU |
關鍵字: | artificial neural network (ANN);explainable artificial intelligence (XAI);local interpretable model-agnostic explanations (LIME);Machine learning;optical emission spectroscopy;plasma-liquid interaction;solution plasma;Chemical analysis;Light emission;Lime;Multilayer neural networks;Emission lines;Linear modeling;Multilayer artificial neural networks;Optical emission spectroscopies (OES);Solution conductivity;Spectral feature;Optical emission spectroscopy | 公開日期: | 2021 | 卷: | 18 | 期: | 12 | 來源出版物: | Plasma Processes and Polymers | 摘要: | This study presents an explainable artificial intelligence (XAI) vision for optical emission spectroscopy (OES) of plasma in aqueous solution. We aim to characterize the plasma and OES with XAI. Trained with 18000 spectra, a multilayer artificial neural network (ANN) model accurately predicted the solution conductivity. Local interpretable model-agnostics explanations (LIME), an XAI method, interpreted the model through perturbing spectral features and fitting the feature contribution with a linear model. LIME showed that OH, Hγ, and Hβ emission lines were critical to the model, differing from the lines typically selected by humans. The results demonstrated that machine captured the spectral features neglected by humans. We believe using XAI for plasma OES analysis impacts the fields of plasma and analytical chemistry. ? 2021 Wiley-VCH GmbH. |
URI: | https://www.scopus.com/inward/record.uri?eid=2-s2.0-85114799300&doi=10.1002%2fppap.202100096&partnerID=40&md5=2ce405072fb40b382f819eec61cbe95c https://scholars.lib.ntu.edu.tw/handle/123456789/598219 |
ISSN: | 16128850 | DOI: | 10.1002/ppap.202100096 |
顯示於: | 化學工程學系 |
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