https://scholars.lib.ntu.edu.tw/handle/123456789/598666
標題: | Particulate matter in a motorcycle-dominated urban area: Source apportionment and cancer risk of lung deposited surface area (LDSA) concentrations | 作者: | Chang P.-K Griffith S.M Chuang H.-C Chuang K.-J Wang Y.-H Chang K.-E Hsiao T.-C. TA-CHIH HSIAO |
關鍵字: | Excess lifetime cancer risk;Lung deposited surface area;Motorcycle;Particle size distribution;PM1;Air pollution;Biological organs;Diseases;Factorization;Light transmission;Morphology;Motorcycles;Particle size;Regression analysis;Size distribution;Area concentrations;Black carbon;Cancer risk;Deposited surface areas;Particle number concentration;Particles-size distributions;Traffic emissions;Particle size analysis;black carbon;particulate organic matter;cancer;particulate matter;source apportionment;surface area;urban area;air pollution;airborne particle;Article;cancer risk;circadian rhythm;concentration (parameter);dangerous goods;lung cancer;motorcycle;particle size;particulate matter 1.0;risk assessment;secondary organic aerosol;Taiwan;traffic and transport;traffic pollution;air pollutant;analysis;environmental monitoring;exhaust gas;human;lung;neoplasm;toxicity;Air Pollutants;Air Pollution;Environmental Monitoring;Humans;Lung;Neoplasms;Particle Size;Particulate Matter;Vehicle Emissions | 公開日期: | 2022 | 卷: | 427 | 來源出版物: | Journal of Hazardous Materials | 摘要: | Source-apportioned particle concentrations are necessary to properly evaluate the health impacts of air pollution. In this study, a measurement station was established at an urban roadside in northern Taiwan to the investigate lung deposited surface area (LDSA) concentration, a relevant metric for the adverse health effects of aerosol exposure, along with PM1 and equivalent black carbon (eBC) concentrations, particle number concentration (PNC), and particle size distribution (PSD). Through positive matrix factorization and multi-linear regression analysis, we attributed 57% of LDSA to traffic emissions over the entire study. During rush hour, the motorcycle fraction increased to 0.83 and LDSA (77.6 ± 9.9 ?m2/cm3) and PNC (14,000 ± 2400 particles/cm3) values peaked, while 74% of LDSA was attributed to traffic. The LDSA ratio, defined as the ratio of measured LDSA to that estimated from the particle size distribution with a spherical assumption, also increased, highlighting the greater degree of fractal morphology during rush hour. The relationship between LDSA emitted by traffic and PNC yielded a higher r2 (0.92) than the r2 between traffic LDSA and eBC (0.82). Finally, the excess lifetime cancer risk linked with traffic emission was 1.56 × 10-4 (i.e. 15.6 excess cancer cases for a population of 100,000 people) based on the LDSA apportionment results. ? 2022 Elsevier B.V. |
URI: | https://www.scopus.com/inward/record.uri?eid=2-s2.0-85123240255&doi=10.1016%2fj.jhazmat.2021.128188&partnerID=40&md5=6638efe7e476309144223560c438137e https://scholars.lib.ntu.edu.tw/handle/123456789/598666 |
ISSN: | 03043894 | DOI: | 10.1016/j.jhazmat.2021.128188 |
顯示於: | 環境工程學研究所 |
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